Three separate laboratory tasks

PHYSICS · Multi-part · Fermi University Physics · Nuclear Physics · Radioactivity and decay modes · Radiation interactions, detection and dosimetry

The Nucleus Resolved, Ch What it is used for: medicine, dating and analysis

Problem

Three separate laboratory tasks, worked in turn. ((a)) A 99Mo/99mTc{}^{99}\mathrm{Mo}/{}^{99m}\mathrm{Tc} generator has a parent activity of 40 GBq40\,\mathrm{GBq} of 99Mo{}^{99}\mathrm{Mo} at the moment it is loaded (freshly eluted, so the daughter starts at zero). Take T1/2(99Mo)=66 hT_{1/2}({}^{99}\mathrm{Mo}) = 66\,\mathrm{h}, T1/2(99mTc)=6.0 hT_{1/2}({}^{99m}\mathrm{Tc}) = 6.0\,\mathrm{h}, and a branching fraction of 87.6 %87.6\,\% of 99Mo{}^{99}\mathrm{Mo} decays feeding the isomer. Calculate the activity of 99mTc{}^{99m}\mathrm{Tc} that is eluted 24 h24\,\mathrm{h} after loading. ((b)) A bone sample has a measured 14C/12C{}^{14}\mathrm{C}/{}^{12}\mathrm{C} ratio equal to 0.150.15 of the modern atmospheric ratio. Take T1/2(14C)=5730 yrT_{1/2}({}^{14}\mathrm{C}) = 5730\,\mathrm{yr}. The sample is known to have derived its carbon from a marine reservoir with an apparent age offset of 400 yr400\,\mathrm{yr} relative to the atmosphere. Calculate the conventional radiocarbon age of the sample corrected for this reservoir effect (no calendar calibration curve is supplied or required). ((c)) A suspect residue is irradiated for 45 min45\,\mathrm{min} in a thermal neutron flux of 8.0×1012 cm−2 s−18.0\times10^{12}\,\mathrm{cm^{-2}\,s^{-1}} to test for gold via 197Au(n,γ)198Au{}^{197}\mathrm{Au}(n,\gamma){}^{198}\mathrm{Au}, with σnγ=98.7 b\sigma_{n\gamma} = 98.7\,\mathrm{b} and T1/2(198Au)=64.8 hT_{1/2}({}^{198}\mathrm{Au}) = 64.8\,\mathrm{h}. Immediately after irradiation the sample is counted for 1.0 h1.0\,\mathrm{h} in the 412 keV412\,\mathrm{keV} line (emitted in 95.6 %95.6\,\% of decays) with a detector of 3.0 %3.0\,\% efficiency for that line. A background count of 2525 counts is recorded in the same 1.0 h1.0\,\mathrm{h} window, and a peak is judged detected only if the net counts exceed 3B3\sqrt{B} above that background, BB being the background count (a simpler and looser rule than Chapter 10's detection limit LD=2.71+4.65BL_D = 2.71 + 4.65\sqrt{B}). Decay of 198Au{}^{198}\mathrm{Au} during the 1.0 h1.0\,\mathrm{h} count may be neglected, since it is only about 1 %1\,\% of the half-life. Calculate the minimum mass of gold detectable under these conditions.

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